Dynamic pore modulation of contracted carbon fiber filter for wastewater treatment: Filtration performance and in-situ regeneration mechanism

作者: Tao Xu, Lin Shi, Senlin Shao, Hui Wang, Yu Huang, Lei Xing, Re Xia, Ruggero Rossi, Liandong Zhu, Hua Zhu, Wulin Yang, Xuhui Mao, Xu Wang

来源出版物: Chemical Engineering Journal 卷:473 文献号：145243 出版年: 1 October 2023摘要: Antifouling and selectivity are the major challenges in membrane separation technologies. Inspired by membranes with tunable pore sizes in filtration systems, we propose a contracted carbon fibrous filter (CCF) with an inversed-triangle structure (ITS) using commercial carbon fibers that can control the filter pore size by adjusting the external force loading. By increasing the force loading on fibers, CCF pores shrunk from 2.02 to 0.98 µm, while maintaining a high rejection efficiency of kaolin particles (>99%) at a water flux ranging from 679.7 to 354.9 L m-2 h−1. The role of the ITS and the filtration mechanism of the carbon fibers was revealed via computational simulations and experimental results. Various cleaning strategies were explored to regenerate CCF performance after fouling. A mean flux recovery of 99.6% could be achieved during the nine-cycle filtration by adjusting the pore size combined with electrocleaning. Additionally, a removal mechanism for internal fouling was proposed. This study demonstrates that the novel CCF provides a simple and reliable strategy for wastewater filtration.

关键词：Wastewater filtration; Contracted carbon fiber; Pore size control; Flux recovery; Antifouling

通讯作者：Xuhui Mao，Xu Wang

影响因子：15.1